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1 article(s) from Hisaeda, Yoshio

Learning from B₁₂ enzymes: biomimetic and bioinspired catalysts for eco-friendly organic synthesis

Keishiro Tahara,
Ling Pan,
Toshikazu Ono and
Yoshio Hisaeda

Beilstein J. Org. Chem. 2018, 14, 2553–2567, doi:10.3762/bjoc.14.232

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Graphical Abstract

Figure 1: (a) Structure and (b) reactivity of B₁₂.

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Figure 2: (a) Schematic representation of B₁₂ enzyme-involving systems. (b) Construction of biomimetic and bi...

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Scheme 1: (a) Carbon-skeleton rearrangement mediated by a coenzyme B₁₂-depenedent enzyme. (b) Electrochemical...

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Scheme 2: Electrochemical carbon-skeleton arrangements mediated by B₁₂ model complexes.

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Figure 3: Key electrochemical reactivity of 1 and 2 in methylated forms.

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Scheme 3: Carbon-skeleton arrangements mediated by B₁₂-vesicle artificial enzymes.

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Scheme 4: Carbon-skeleton arrangements mediated by B₁₂-HSA artificial enzymes.

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Scheme 5: Photochemical carbon-skeleton arrangements mediated by B₁₂-Ru@MOF.

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Scheme 6: (a) Methyl transfer reaction mediated by B₁₂-dependent methionine synthase. (b) Methyl transfer rea...

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Scheme 7: Methyl transfer reaction for the detoxification of inorganic arsenics.

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Scheme 8: (a) Dechlorination of 1,1,2,2-tetrarchloroethene mediated by a reductive dehalogenase. (b) Electroc...

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Scheme 9: Visible-light-driven dechlorination of DDT using 1 in the presence of photosensitizers.

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Scheme 10: 1,2-Migration of a phenyl group mediated by the visible-light-driven catalytic system composed of 1...

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Scheme 11: Ring-expansion reactions mediated by the B₁₂-TiO₂ hybrid catalyst with UV-light irradiation.

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Scheme 12: Trifluoromethylation and perfluoroalkylation of aromatic compounds achieved through electrolysis wi...

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Published 02 Oct 2018

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Learning from B12 enzymes: biomimetic and bioinspired catalysts for eco-friendly organic synthesis

Learning from B₁₂ enzymes: biomimetic and bioinspired catalysts for eco-friendly organic synthesis